Entanglement is a strange phenomenon in quantum physics where two particles are inherently connected to each other no matter the distance between them. When one is measured, the other measurement is instantly a given. Researchers from Purdue University have proposed a novel, unconventional approach to generate a special light source made up of entangled photons. On Sept. 6, 2022, they published their findings in Physical Review Research.
The team proposed a method to generate entangled photons at extreme-ultraviolet (XUV) wavelengths where no such source currently exists. Their work provides a road map on how to generate these entangled photons and use them to track the dynamics of electrons in molecules and materials on the incredibly short timescales of attoseconds.
“The entangled photons in our work are guaranteed to arrive at a given location within a very short duration of attoseconds, as long as they travel the same distance,” says Dr. Niranjan Shivaram, assistant professor of Physics and Astronomy. “This correlation in their arrival time makes them very useful to measure ultrafast events. One important application is in attosecond metrology to push the limits of measurement of the shortest time scale phenomena. This source of entangled photons can also be used in quantum imaging and spectroscopy, where entangled photons have been shown to enhance the ability to gain information, but now at XUV and even X-ray wavelengths.”
The authors of the publication, titled “Attosecond entangled photons from two-photon decay of metastable atoms: A source for attosecond experiments and beyond,” are all from the Purdue University Department of Physics and Astronomy and work with the Purdue Quantum Science and Engineering Institute (PQSEI). They are Dr. Yimeng Wang, recent graduate of Purdue University; Siddhant Pandey, PhD candidate in the field of experimental ultrafast spectroscopy; Dr. Chris H. Greene, Albert Overhauser Distinguished Professor of Physics and Astronomy; and Dr. Shivaram.
“The Department of Physics and Astronomy at Purdue has a strong atomic, molecular and optical (AMO) physics program, which brings together experts in various subfields of AMO,” says Shivaram. “Chris Greene’s expert knowledge of theoretical atomic physics combined with Niranjan’s background in the relatively young field of experimental attosecond science led to this collaborative project. While many Universities have AMO programs, Purdue’s AMO program is uniquely diverse in that it has experts in multiple subfields of AMO science.”
Each researcher played a significant role in this ongoing research. Greene initially suggested the idea of using photons emitted by helium atoms as a source of entangled photons and Shivaram suggested applications to attosecond science and proposed experimental schemes. Wang and Greene then developed the theoretical framework to calculate entangled photon emission from helium atoms, while Pandey and Shivaram made estimates of entangled photon emission/absorption rates and worked out the details of the proposed attosecond experimental schemes.
The publication marks the beginning of this research for Shivaram and Greene. In this publication, the authors propose the idea and work out the theoretical aspects of the experiment. Shivaram and Greene plan to continue to collaborate on experimental and further theoretical ideas. Shivaram’s lab, the Ultrafast Quantum Dynamics Group, is currently building an apparatus to experimentally demonstrate some of these ideas. According to Shivaram, the hope is that other researchers in attosecond science will begin working on these ideas. A concerted effort by many research groups could further increase the impact of this work. Eventually, they hope to get the timescale of entangled photons down to the zeptosecond, 10-21 seconds.
“Typically, experiments on attosecond timescales are performed using attosecond laser pulses as ‘strobes’ to ‘image’ the electrons. Current limits on these pulses are around 40 attoseconds. Our proposed idea of using entangled photons could push this down to a few attoseconds or zeptoseconds,” says Shivaram.
In order to understand the timing, one must understand that electrons play a fundamental role in determining the behavior of atoms, molecules and solid materials. The timescale of motion of electrons is typically in the femtosecond (one millionth of a billionth of a second – 10-15 seconds) and attosecond (one billionth of a billionth of a second, or 10-18 seconds) scale. According to Shivaram, gaining insight into the dynamics of electrons and tracking their motion on these ultrashort timescales is essential.
“The goal of the field of ultrafast science is to make such ‘movies’ of electrons and then use light to control the behavior of these electrons to engineer chemical reactions, make materials with novel properties, make molecular-scale devices, etc.,” he says. “This is light-matter interaction at its most basic level, and the possibilities for discovery are many. A single zeptosecond is 10-21 seconds. A thousand zeptoseconds is an attosecond. Researchers are only now beginning to explore zeptosecond phenomena, though it is experimentally out of reach due to lack of zeptosecond laser pulses. Our unique approach of using entangled photons instead of photons in laser pulses could allow us to reach the zeptosecond regime. This will require considerable experimental effort and is likely possible on the timescale of five years.”
About the Department of Physics and Astronomy at Purdue University
Purdue Department of Physics and Astronomy has a rich and long history dating back to 1904. Our faculty and students are exploring nature at all length scales, from the subatomic to the macroscopic and everything in between. With an excellent and diverse community of faculty, postdocs, and students who are pushing new scientific frontiers, we offer a dynamic learning environment, an inclusive research community, and an engaging network of scholars.
Physics and Astronomy is one of the seven departments within the Purdue University College of Science. World-class research is performed in astrophysics, atomic and molecular optics, accelerator mass spectrometry, biophysics, condensed matter physics, quantum information science, particle and nuclear physics. Our state-of-the-art facilities are in the Physics Building, but our researchers also engage in interdisciplinary work at Discovery Park District at Purdue, particularly the Birck Nanotechnology Center and the Bindley Bioscience Center. We also participate in global research including at the Large Hadron Collider at CERN, Argonne National Laboratory, Brookhaven National Laboratory, Fermilab, the Stanford Linear Accelerator, the James Webb Space Telescope, and several observatories around the world.
About Purdue University
Purdue University is a top public research institution developing practical solutions to today’s toughest challenges. Ranked in each of the last four years as one of the 10 Most Innovative universities in the United States by U.S. News & World Report, Purdue delivers world-changing research and out-of-this-world discovery. Committed to hands-on and online, real-world learning, Purdue offers a transformative education to all. Committed to affordability and accessibility, Purdue has frozen tuition and most fees at 2012-13 levels, enabling more students than ever to graduate debt-free. See how Purdue never stops in the persistent pursuit of the next giant leap at https://stories.purdue.edu.
Writer: Cheryl Pierce, Communications Specialist
Contributor: Dr. Niranjan Shivaram, Assistant Professor of Physics and Astronomy
Graphic by: Cheryl Pierce with elements from Adobe Stock
Physical Review Research
Attosecond entangled photons from two-photon decay of metastable atoms: A source for attosecond experiments and beyond
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