Oxide interfaces put new twist on electron spins
Interfaces made by stacking certain complex oxide materials can tune the quantum interactions between electrons, yielding exotic spin textures
DOE/US Department of Energy
In magnetic solids, electrons feel each other as what scientists call an effective magnetic field. This field forces the electrons’ magnetic moments (spins) to align. If the arrangement of atoms is not fully symmetric, an additional magnetic force known as Dzyaloshinskii-Moriya Interaction (DMI) can emerge. DMI forces the spins to reorient and form whirling patterns called skyrmions. Using very careful synthesis methods, researchers joined two different materials, lanthanum manganite (LaMnO3) and strontium iridium oxide (SrIrO3), with atomic precision. The resulting interfaces support DMI, thus enabling skyrmion generation. These findings provide insight into the nature of DMIs creating textures with a special type of asymmetry called chirality. They also highlight the emergence of interface-driven topological phenomena.
Skyrmions have dimensions in the nanometer range and behave like particles that can be moved using small electric currents. This means information stored using skyrmions can be manipulated with very small power consumption. Skyrmions are also very resistant against external influences such as temperature and vibrations. Consequently, scientists believe that skyrmions can be used for ultra-high-density information storage devices. The latter will enable devices to encode much larger amounts of data than current computer hard disks.
Skyrmions can be created by combining two ingredients necessary for DMI to emerge. The first ingredient is lack of inversion symmetry. When dissimilar materials A and B are joined, one creates a system without inversion symmetry. Inverting atom A (or B) with respect to the interface plane produces a different system. The second ingredient calls for electron spins that are strongly influenced by the electron motion around the nucleus. This interaction is called spin-orbit coupling and develops in materials with heavy atoms.
Researchers at Oak Ridge National Laboratory combined the two ingredients by stacking LaMnO3 and SrIrO3 in a manner that aligns the atoms and their orbitals. They “observed” skyrmions through their signature electrical response known as Topological Hall Effect (THE). In THE, an electrical current that crosses the skyrmions experiences an emergent magnetic field, and is deflected sideways, although no external magnetic field is present. By changing the order of each atomic layer, researchers were able to maximize the interface asymmetry and thus the DMI strength, which in turn inferred the creation of smaller and denser skyrmions. This result shows that interfaces can effectively tune DMI strength and tailor skyrmions size to application requirements.
This work was supported by the Department of Energy (DOE) Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. Use of the Advanced Photon Source and the Advanced Light Source, both of which are DOE Office of Science user facilities, was supported by DOE’s Office of Science. The Hall effect measurements in high magnetic fields were performed at the National High Magnetic Field Laboratory, which is supported by the National Science Foundation.
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